FotR: The Shadow of the Past and The Council of Elrond (sorry, had to go for two) - I love the way the story builds up and the connections with the events of the Hobbit are established.
TTT: Helm's Deep - My favourite chapter from when I first read LotR, a great description of a seemingly hopeless battle and wonderfully resolved.
RotK: The Scouring of the Shire - As someone said, Merry and Pippin come into their own.
The Silm: Of Turin Turambar - Tragic and heroic.
The Hobbit: Inside Information - Just recently read that chapter again. The interplay between Bilbo and Smaug, and the development of Smaug's character, are so enjoyable.
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Do you mind? I'm busy doing the fishstick. It's a very delicate state of mind!
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