As Gandalf said, Sauron was calling all evil things to him in Mordor. As Smeagol (and Sam and Frodo) got closer and closer to Barad-dur, more and more of Gollum came out. It became harder and harder for Smeagol to be "nice" to Frodo and Sam, and not betray them, as his Gollum personality took over more often.
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But Melkor also was there, and he came to the house of Fëanor, and there he slew Finwë King of the Noldor before his doors, and spilled the first blood in the Blessed Realm; for Finwë alone had not fled from the horror of the Dark.
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